CiteULike: dchen Bonn

Flow of Wet Granular Materials

N Huang — 2008-06-22T00:55:36-00:00

Physical Review Letters, Vol. 94, No. 2. (2005)

The transition from frictional to lubricated flows of a dense suspension of non-Brownian particles is studied. The pertinent parameter characterizing this transition is the Leighton number Le = , the ratio of lubrication to frictional forces. Le defines a critical shear rate below which no steady flow without localization exists. In the frictional regime the shear flow is localized. The lubricated regime is not simply viscous: the ratio of shear to normal stresses remains constant and the velocity profile has a universal form in both frictional and lubricated regimes. Finally, a discrepancy between local and global measurements of viscosity is identified, which suggests inhomogeneity of the material under flow.

Transition from a simple yield-stress fluid to a thixotropic material

A Ragouilliaux — 2008-06-10T16:55:47-00:00

Physical Review E (Statistical, Nonlinear, and Soft Matter Physics), Vol. 76, No. 5. (2007)

From magnetic resonance imaging rheometry we show that a pure emulsion can be turned from a simple yield stress fluid to a thixotropic material by adding a small fraction of colloidal particles. The two fluids have the same behavior in the liquid regime but the loaded emulsion exhibits a critical shear rate below which no steady flows can be observed. For a stress below the yield stress, the pure emulsion abruptly stops flowing, whereas the viscosity of the loaded emulsion continuously increases in time, which leads to an apparent flow stoppage. This phenomenon can be very well represented by a model assuming a progressive increase of the number of droplet links via colloidal particles.

Kinetics of ergodic-to-nonergodic transitions in charged colloidal suspensions: Aging and gelation

Hajime Tanaka — 2008-05-13T15:20:47-00:00

Physical Review E (Statistical, Nonlinear, and Soft Matter Physics), Vol. 71, No. 2. (2005)

There are two types of isotropic disordered nonergodic states in colloidal suspensions: colloidal glasses and gels. In a recent paper [H. Tanaka, J. Meunier, and D. Bonn, Phys. Rev. E 69, 031404 (2004)], we discussed the static aspect of the differences and the similarities between the two. In this paper, we focus on the dynamic aspect. The kinetics of the liquid-glass transition is called "aging," while that of the sol-gel transition is called "gelation." The former is primarily governed by repulsive interactions between particles, while the latter is dominated by attractive interactions. Slowing down of the dynamics during aging reflects the increasing cooperativity required for the escape of a particle from the cage formed by the surrounding particles, while that during gelation reflects the increase in the size of particle clusters towards the percolation transition. Despite these clear differences in the origin of the slowing down of the kinetics between the two, it is not straightforward experimentally to distinguish them in a clear manner. For an understanding of the universal nature of ergodic-to-nonergodic transitions, it is of fundamental importance to elucidate the differences and the similarities in the kinetics between aging and gelation. We consider this problem, taking Laponite suspension as an explicit example. In particular, we focus on the two types of nonergodic states: (i) an attractive gel formed by van der Waals attractions for high ionic strengths and (ii) a repulsive Wigner glass stabilized by long-range Coulomb repulsions for low ionic strengths. We demonstrate that the aging of colloidal Wigner glass crucially differs not only from gelation, but also from the aging of structural and spin glasses. The aging of the colloidal Wigner glass is characterized by the unique cage-forming regime that does not exist in the aging of spin and structural glasses.

Laponite: Aging and Shear Rejuvenation of a Colloidal Glass

Daniel Bonn — 2008-04-25T23:08:28-00:00

Physical Review Letters, Vol. 89, No. 1. (13 June 2002), 015701.

Fluctuation-Dissipation Theorem in an Aging Colloidal Glass

Sara Farouji — 2007-11-26T20:20:36-00:00

Physical Review Letters, Vol. 98, No. 10. (2007)

We provide a direct experimental test of the fluctuation-dissipation theorem (FDT) in an aging colloidal glass. The use of combined active and passive microrheology allows us to independently measure both the correlation and response functions in this nonequilibrium situation. Contrary to previous reports, we find no deviations from the FDT over several decades in frequency (1 Hz–10 kHz) and for all aging times. In addition, we find two distinct viscoelastic contributions in the aging glass, including a nearly elastic response at low frequencies that grows during aging.

Shear Thickening of Cornstarch Suspensions as a Reentrant Jamming Transition

Abdoulaye Fall — 2008-03-18T01:32:20-00:00

Physical Review Letters, Vol. 100, No. 1. (2008)

We study the rheology of cornstarch suspensions, a non-Brownian particle system that exhibits shear thickening. From magnetic resonance imaging velocimetry and classical rheology it follows that as a function of the applied stress the suspension is first solid (yield stress), then liquid, and then solid again when it shear thickens. For the onset of thickening we find that the smaller the gap of the shear cell, the lower the shear rate at which thickening occurs. Shear thickening can then be interpreted as the consequence of dilatancy: the system under flow wants to dilate but instead undergoes a jamming transition because it is confined, as confirmed by measurement of the dilation of the suspension as a function of the shear rate.